There are many special road and places to see in Northwest Argentina, plus it is the main, but not necessarily the most interesting way to go to Bolivia
At that Bolivian border there are 5121 Km to Ushuaia.
A very interesting road and town is IRUYA. Look closely at your map and you will see that it is northeast going north.
In Jujuy, the best motorcycle place is the Honda dealer. His website is listed below:
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